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To solve a similar problem (plasterboard butting up not very flush to an aluminium frame), I used angled pine moulding / beading.
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I'll post some more pics as I'm struggling to work out your suggestion.
The issue is the frame is wood and you can't plaster on top of it.
Here is a birds eye view of the issue.
At the moment the wood frame is flush. But after the skim it'll be too low.