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you can probably pick up Dark Arts in their Aries popup at the moment (not sure when its ending). Coborn coffee are also based near Kensal Rise but not sure about local pickup. Plenty of 'proper' coffee shops also stock a wide range of great beans, Batch Baby in east or Prufrock on leather lane. Monmouth or even Algerian Coffee Stores are central if you arent fussed about light roasts
Anyone can recommend any central-ish London-based roasters? Have a coffee subscription from Django but occasionally use that up before I get a new bag and want an option for when I need another bag on an ad hoc basis and don't want to pay 3.50 for postage if I can just pop by a shop instead.. Ozone and Square Mile are my go-tos but haven't been looking around for quite a while!