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https://montanasvacias.com/spanishdivide/ which goes from Delta d'Ebro to
That one looks great. And has the benefit you could get the train out to Tortosa near the start, buy a gravel bike from the Decathlon there to ride it and get the ferry back from Bilbao, meaning no air travel required.
I'd need to have a look where the Europe Divide goes (https://europeandividetrail.com/)
https://www.komoot.com/collection/1070173/7-600-km-across-the-continent-european-divide-trail
There's some other "Spanish divide" routes I've been eyeballing...
https://iberica-traversa.com/ whch goes SE from Irun to Tarifa
https://montanasvacias.com/spanishdivide/ which goes from Delta d'Ebro to