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Ta. Problem with those two countries is that I've ridden around both of them already and I'm running out of Belgian beers that I've not tried :)
The ISR just seems like extra paperwork for something I already do so isn't particularly appealing. I need awards/goals to encourage me to ride, not more admin.
Ultra is 1 per year, so I can't stack them and get it any quicker "Established in 1998 for those who complete 10 Super Randonneur series. Only one series per year counts, and the series do not have to be consecutive."
There are some nice looking Dutch and Belgian audaxes, some starting and finishing pretty near ferries [+ breweries], that look quite appealing, for something different and logistically fairly easy. There are threads on YACF.