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I think Fenton House is slightly closer but according to their listing neither have food & drink. George Inn is the closest with listed food & drink but may not take NT vouchers for payment. I've only ever visited Osterley Park once, and that was for a meeting, so that would be good but the obvious route is no fun at all. A back lane route to the Ashridge Estate could be good.
That's quite a nice idea but there aren't any obvious destinations starting from North London. I shall look at their list of coffee shops some more.