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I did that in reverse a couple of years ago. I don't have a specific route but I can recommend the section of http://www.viasverdes.com/mapas_en.asp going west out of Girona and the bit going into San Sebastian.
There's also an old edscoble thread that details a route through the west part of the Pryennes (going into France if I remember correctly)...
RubberDucky
Anyone got any tips for routing between Girona and Bilbao? Wouldn't mind doing a mountain pass. Got around 9 days to play with.