They will feel different of course but I think the feel of steel is romanticised. With a carbon fork, deep wheels, high tyre pressure, it could feel very stiff.
The bigger differences will come from other things but including geometry and construction as c00ps says. A manufacturer can make a comfortable alloy frame or a stiff one using tubing shapes, tube wall thicknesses and geometry. See for example Cannondale Synapse vs Cannondale CAAD of a few years ago.
It would be difficult to compare two frame's comfort or feel unless they're very similar bikes and the material is the only difference.
They will feel different of course but I think the feel of steel is romanticised. With a carbon fork, deep wheels, high tyre pressure, it could feel very stiff.
The bigger differences will come from other things but including geometry and construction as c00ps says. A manufacturer can make a comfortable alloy frame or a stiff one using tubing shapes, tube wall thicknesses and geometry. See for example Cannondale Synapse vs Cannondale CAAD of a few years ago.
It would be difficult to compare two frame's comfort or feel unless they're very similar bikes and the material is the only difference.