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I don't have anything helpful to say, but I am interested to know what you eventually find as the solution. I have a very similar situation around the door frame of our side entrance.
I am afraid to tackle it as I worry it will end up being a can of worms when I start to chip away - that the small patch that is visibly damaged now becomes a huge area that falls off.
Looks like it could have been poorly mixed too. It's not uncommon where there's no room for expansion/contraction that a small crack opens up, water gets in, freezes and expands the crack then stays wet and eventually destroys the mortar. There would normally be some kind of frame sealant to help avoid that.
A little shrunken head would look great in that hole though.