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Oh, hang on you mean it won't go from second highest to highest, even though the cable is slack? Have you tried opening up the H limit screw? Sometimes it can get close but not close enough to complete the shift.
Also, eyeball or tighten the cassette to make sure the cassette cogs all have the same gap and it's not loose.
@Dammit
When you say 'down' do you mean into a higher or lower gear?
Assuming mechanical?
Does pulling the cable (at the downtube say) without the shifter change properly?
If it's not going into higher gears, it's not releasing cable so something is sticking - either shifter or the cable.