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edscoble
I rode West to East last year and loved it.
I'm kinda oldskool so don't have an online route but I've got some photos online here with the points I went through. I loved the whole thing but some highlights include the route from Jaca to Ainsa (via 3011 and the A1604) and the gorge north of Campo (N260).
There's also the Vias Verdes (which I have LFGSS to thank for) which has a couple of applicable sections for you. I loved the one from Irun headed south and Olat to Girona.
Finally there's Ed's account of the first half of his trip from Santander to Perpignan here: https://www.lfgss.com/conversations/254424/
Hope that helps, any specific questions just shout/pm