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It's a wee bit tricky to get the splatter effect; one way to explain it is that I'm rocking the nozzle backwards off its axis (forcing the paint to come out unevenly) with my thumb after initially spraying away from the surface, which seems counter-intuitive at first but works with practice. The pocket Spray.Bike cans seem to coat a lot thicker than the larger ones, so the surface of what you're painting will be egg-shelled if using this technique.
following closely! hoping to do a spray. bike job on a frame soon, though probably less ambitious than yours. how are you getting that mist/splatter effect you can see really clearly on the stem and bars?