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I've always enjoyed Cafe Oberholz for a coffee when in Berlin.
http://www.sanktoberholz.de/?page_id=2957&lang=enIf you want a slightly more off the beaten path sight, check out the Soviet War Memorial in Treptower Park, and while you are out east, have a coffee in Cafe Sibylle on Karl-Marx-Allee (which is also a tiny museum).
http://www.cafe-sibylle-berlin.de/
Doctor_Cake
Brilliant tips, thanks so much! I'm going to stuff my face :)